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2011


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Quantum-Cascade Laser-Based Vibrational Circular Dichroism

Luedeke, S., Pfeifer, M., Fischer, P.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 133(15):5704-5707, 2011 (article)

Abstract
Vibrational circular dichroism (VCD) spectra were recorded with a tunable external-cavity quantum-cascade laser (QCL). In comparison with standard thermal light sources in the IR, QCLs provide orders of magnitude more power and are therefore promising for VCD studies in strongly absorbing solvents. The brightness of this novel light source is demonstrated with VCD and IR absorption measurements of a number of compounds, including proline in water.

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DOI [BibTex]

2011


DOI [BibTex]


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Actively coupled cavity ringdown spectroscopy with low-power broadband sources

Petermann, C., Fischer, P.

OPTICS EXPRESS, 19(11):10164-10173, 2011 (article)

Abstract
We demonstrate a coupling scheme for cavity enhanced absorption spectroscopy that makes use of an intracavity acousto-optical modulator to actively switch light into (and out of) a resonator. This allows cavity ringdown spectroscopy (CRDS) to be implemented with broadband nonlaser light sources with spectral power densities of less than 30 mu W/nm. Although the acousto-optical element reduces the ultimate detection limit by introducing additional losses, it permits absorptivities to be measured with a high dynamic range, especially in lossy environments. Absorption measurements for the forbidden transition of gaseous oxygen in air at similar to 760nm are presented using a low-coherence cw-superluminescent diode. The same setup was electronically configured to cover absorption losses from 1.8 x 10(-8)cm(-1) to 7.5\% per roundtrip. This could be of interest in process analytical applications. (C) 2011 Optical Society of America

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DOI [BibTex]

DOI [BibTex]


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Magnetically actuated propulsion at low Reynolds numbers: towards nanoscale control

Fischer, P., Ghosh, A.

NANOSCALE, 3(2):557-563, 2011 (article)

Abstract
Significant progress has been made in the fabrication of micron and sub-micron structures whose motion can be controlled in liquids under ambient conditions. The aim of many of these engineering endeavors is to be able to build and propel an artificial micro-structure that rivals the versatility of biological swimmers of similar size, e. g. motile bacterial cells. Applications for such artificial ``micro-bots'' are envisioned to range from microrheology to targeted drug delivery and microsurgery, and require full motion-control under ambient conditions. In this Mini-Review we discuss the construction, actuation, and operation of several devices that have recently been reported, especially systems that can be controlled by and propelled with homogenous magnetic fields. We describe the fabrication and associated experimental challenges and discuss potential applications.

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Video - Nanospropellers DOI [BibTex]


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The Oxidation of Fe(111)

Davies, R., Edwards, D., Gräfe, J., Gilbert, L., Davies, P., Hutchings, G., Bowker, M.

Surface Science, 605(17-18):1754-1762, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Weak value amplified optical activity measurements

Pfeifer, M., Fischer, P.

Opt. Express, 19(17):16508-16517, OSA, 2011 (article)

Abstract
We present a new form of optical activity measurement based on a modified weak value amplification scheme. It has recently been shown experimentally that the left- and right-circular polarization components refract with slightly different angles of refraction at a chiral interface causing a linearly polarized light beam to split into two. By introducing a polarization modulation that does not give rise to a change in the optical rotation it is possible to differentiate between the two circular polarization components even after post-selection with a linear polarizer. We show that such a modified weak value amplification measurement permits the sign of the splitting and thus the handedness of the optically active medium to be determined. Angular beam separations of Δθ ∼ 1 nanoradian, which corresponds to a circular birefringence of Δn ∼ 1 × 10−9, could be measured with a relative error of less than 1%.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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High-resolution x-ray absorption spectroscopy of BaTiO_3: Experiment and first-principles calculations

Chassé, A., Borek, S., Schindler, K., Trautmann, M., Huth, M., Steudel, F., Makhova, L., Gräfe, J., Denecke, R.

Physical Review B, 84, pages: 195135, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Ferromagnetism of ZnO influenced by physical and chemical treatment

Chen, Y.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Herstellung und Charakterisierung von ultradünnen, funktionellen CoFeB Filmen

Streckenbach, F.

Hochschule Esslingen / Hochschule Aalen, Esslingen / Aalen, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Hydrogen adsorption on metal-organic frameworks

Streppel, B.

Universität Stuttgart, Stuttgart, 2011 (phdthesis)

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link (url) [BibTex]

link (url) [BibTex]


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Electron theory of fast and ultrafast dissipative magnetization dynamics

Fähnle, M., Illg, C.

{Journal of Physics: Condensed Matter}, 23, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Large-area hard magnetic L10-FePt nanopatterns by nanoimprint lithography

Bublat, T., Goll, D.

{Nanotechnology}, 22(31), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Hydrogen storage by cryoadsorption in ultrahigh-porosity metal-organic frameworks

Hirscher, M.

{Angewandte Chemie International Edition}, 50(3):581-582, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Amorphous grain boundary layers in the ferromagnetic nanograined ZnO films

Straumal, B. B., Mazilkin, A. A., Protasova, S. G., Myatiev, A. A., Straumal, P. B., Goering, E., Baretzky, B.

In 520, pages: 1192-1194, Hersonissos, Greece, 2011 (inproceedings)

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DOI [BibTex]

DOI [BibTex]


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Multilayer Fresnel zone plate for soft X-ray microscopy resolves sub-39 nm structures

Mayer, M., Grévent, C., Szeghalmi, A., Knez, M., Weigand, M., Rehbein, S., Schneider, G., Baretzky, B., Schütz, G.

{Ultramicroscopy}, 111, pages: 1706-1711, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Generalized Gilbert equation including inertial damping: derivation from an extended breathing Fermi surface model

Fähnle, M., Steiauf, D., Illg, C.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]


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Hydrogen physisorption in high SSA microporous materials - A comparison between AX-21\textunderscore33 and MOF-177 at cryogenic conditions

Schlichtenmayer, M., Streppel, B., Hirscher, M.

{International Journal of Hydrogen Energy}, 36, pages: 586-591, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Inversed solid-phase grain boundary wetting in the Al-Zn system

Protasova, S. G., Kogtenkova, O. A., Straumal, B. B., Zieba, P., Baretzky, B.

In 46, pages: 4349-4353, Mie, Japan, 2011 (inproceedings)

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DOI [BibTex]

DOI [BibTex]


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Magnetic vortex core reversal by excitation of spin waves

Kammerer, M., Weigand, M., Curcic, M., Noske, M., Sproll, M., Vansteenkiste, A., Van Waeyenberge, B., Stoll, H., Woltersdorf, G., Back, C. H., Schütz, G.

{Nature Communications}, 2, pages: 279-284, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Toward simple control for complex, autonomous robotic applications: combining discrete and rhythmic motor primitives

Degallier, S., Righetti, L., Gay, S., Ijspeert, A.

Autonomous Robots, 31(2-3):155-181, October 2011 (article)

Abstract
Vertebrates are able to quickly adapt to new environments in a very robust, seemingly effortless way. To explain both this adaptivity and robustness, a very promising perspective in neurosciences is the modular approach to movement generation: Movements results from combinations of a finite set of stable motor primitives organized at the spinal level. In this article we apply this concept of modular generation of movements to the control of robots with a high number of degrees of freedom, an issue that is challenging notably because planning complex, multidimensional trajectories in time-varying environments is a laborious and costly process. We thus propose to decrease the complexity of the planning phase through the use of a combination of discrete and rhythmic motor primitives, leading to the decoupling of the planning phase (i.e. the choice of behavior) and the actual trajectory generation. Such implementation eases the control of, and the switch between, different behaviors by reducing the dimensionality of the high-level commands. Moreover, since the motor primitives are generated by dynamical systems, the trajectories can be smoothly modulated, either by high-level commands to change the current behavior or by sensory feedback information to adapt to environmental constraints. In order to show the generality of our approach, we apply the framework to interactive drumming and infant crawling in a humanoid robot. These experiments illustrate the simplicity of the control architecture in terms of planning, the integration of different types of feedback (vision and contact) and the capacity of autonomously switching between different behaviors (crawling and simple reaching).

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Learning Force Control Policies for Compliant Manipulation

Kalakrishnan, M., Righetti, L., Pastor, P., Schaal, S.

In 2011 IEEE/RSJ International Conference on Intelligent Robots and Systems, pages: 4639-4644, IEEE, San Francisco, USA, sep 2011 (inproceedings)

Abstract
Developing robots capable of fine manipulation skills is of major importance in order to build truly assistive robots. These robots need to be compliant in their actuation and control in order to operate safely in human environments. Manipulation tasks imply complex contact interactions with the external world, and involve reasoning about the forces and torques to be applied. Planning under contact conditions is usually impractical due to computational complexity, and a lack of precise dynamics models of the environment. We present an approach to acquiring manipulation skills on compliant robots through reinforcement learning. The initial position control policy for manipulation is initialized through kinesthetic demonstration. We augment this policy with a force/torque profile to be controlled in combination with the position trajectories. We use the Policy Improvement with Path Integrals (PI2) algorithm to learn these force/torque profiles by optimizing a cost function that measures task success. We demonstrate our approach on the Barrett WAM robot arm equipped with a 6-DOF force/torque sensor on two different manipulation tasks: opening a door with a lever door handle, and picking up a pen off the table. We show that the learnt force control policies allow successful, robust execution of the tasks.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Control of legged robots with optimal distribution of contact forces

Righetti, L., Buchli, J., Mistry, M., Schaal, S.

In 2011 11th IEEE-RAS International Conference on Humanoid Robots, pages: 318-324, IEEE, Bled, Slovenia, 2011 (inproceedings)

Abstract
The development of agile and safe humanoid robots require controllers that guarantee both high tracking performance and compliance with the environment. More specifically, the control of contact interaction is of crucial importance for robots that will actively interact with their environment. Model-based controllers such as inverse dynamics or operational space control are very appealing as they offer both high tracking performance and compliance. However, while widely used for fully actuated systems such as manipulators, they are not yet standard controllers for legged robots such as humanoids. Indeed such robots are fundamentally different from manipulators as they are underactuated due to their floating-base and subject to switching contact constraints. In this paper we present an inverse dynamics controller for legged robots that use torque redundancy to create an optimal distribution of contact constraints. The resulting controller is able to minimize, given a desired motion, any quadratic cost of the contact constraints at each instant of time. In particular we show how this can be used to minimize tangential forces during locomotion, therefore significantly improving the locomotion of legged robots on difficult terrains. In addition to the theoretical result, we present simulations of a humanoid and a quadruped robot, as well as experiments on a real quadruped robot that demonstrate the advantages of the controller.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Learning Motion Primitive Goals for Robust Manipulation

Stulp, F., Theodorou, E., Kalakrishnan, M., Pastor, P., Righetti, L., Schaal, S.

In IEEE/RSJ International Conference on Intelligent Robots and Systems, pages: 325-331, IEEE, San Francisco, USA, sep 2011 (inproceedings)

Abstract
Applying model-free reinforcement learning to manipulation remains challenging for several reasons. First, manipulation involves physical contact, which causes discontinuous cost functions. Second, in manipulation, the end-point of the movement must be chosen carefully, as it represents a grasp which must be adapted to the pose and shape of the object. Finally, there is uncertainty in the object pose, and even the most carefully planned movement may fail if the object is not at the expected position. To address these challenges we 1) present a simplified, computationally more efficient version of our model-free reinforcement learning algorithm PI2; 2) extend PI2 so that it simultaneously learns shape parameters and goal parameters of motion primitives; 3) use shape and goal learning to acquire motion primitives that are robust to object pose uncertainty. We evaluate these contributions on a manipulation platform consisting of a 7-DOF arm with a 4-DOF hand.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Inverse Dynamics Control of Floating-Base Robots with External Constraints: a Unified View

Righetti, L., Buchli, J., Mistry, M., Schaal, S.

In 2011 IEEE International Conference on Robotics and Automation, pages: 1085-1090, IEEE, Shanghai, China, 2011 (inproceedings)

Abstract
Inverse dynamics controllers and operational space controllers have proved to be very efficient for compliant control of fully actuated robots such as fixed base manipulators. However legged robots such as humanoids are inherently different as they are underactuated and subject to switching external contact constraints. Recently several methods have been proposed to create inverse dynamics controllers and operational space controllers for these robots. In an attempt to compare these different approaches, we develop a general framework for inverse dynamics control and show that these methods lead to very similar controllers. We are then able to greatly simplify recent whole-body controllers based on operational space approaches using kinematic projections, bringing them closer to efficient practical implementations. We also generalize these controllers such that they can be optimal under an arbitrary quadratic cost in the commands.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Piezo driven strain effects on magneto-crystalline anisotropy

Badr, E.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Magnetooptische Untersuchungen an granularen und beschichteten MgB2 Filmen

Stahl, C.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Mikromagnetismus der Wechselwirkung von Spinwellen mit Domänenwänden in Ferromagneten

Macke, S.

Universität Stuttgart, Stuttgart, 2011 (phdthesis)

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[BibTex]

[BibTex]


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Magnetism studied with circularly polarized X-rays

Schütz, G., Goering, E., Stoll, H.

{International Journal of Materials Research}, 102(7):773-783, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Coupled vortex oscillations in spatially separated permalloy squares

Vogel, A., Kamionka, T., Martens, M., Drews, A., Chou, K., Tyliszczak, T., Stoll, H., Van Waeyenberge, B., Meier, G.

{Physical Review Letters}, 106, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Contruction of basis functions with crystal symmetry for the spin-cluster expansion of the magnetic energy on the atomic scale

Dietermann, F., Singer, R., Fähnle, M.

{Journal of Mathematical Physics}, 52, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic patterning perpendicular anisotropy FePd alloy films by masked ion irradiation

Merkel, D. G., Bottyán, L., Tanczikó, F., Zolnai, Z., Nagy, N., Vértesy, G., Waizinger, J., Bommer, L.

{Journal of Applied Physics}, 109(12), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Characterization of hydrogen/deuterium adsorption sites in nanoporous Cu-BTC by low-temperature thermal-desorption mass spectroscopy

Krkljus, I., Hirscher, M.

{Microporous and Mesoporous Materials}, 142, pages: 725-729, 2011 (article)

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DOI [BibTex]


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Stability of the current-carrying state in nonhomogeneous MgB2 films

Treiber, S., Stahl, C., Schütz, G., Albrecht, J.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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First measurement of the heat effect of the grain boundary wetting phase transition

Straumal, B. B., Kogtenkova, O. A., Protasova, S. G., Zieba, P., Czeppe, T., Baretzky, B., Valiev, R. Z.

In 46, pages: 4243, Mie, Japan, 2011 (inproceedings)

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DOI [BibTex]

DOI [BibTex]


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Orbital reflectometry of oxide heterostructures

Benckiser, E., Haverkort, M. W., Brück, S., Goering, E., Macke, S., Fraño, A., Yang, X., Andersen, O. K., Cristiani, G., Habermeier, H., Boris, A. V., Zegkinoglou, I., Wochner, P., Kim, H., Hinkov, V., Keimer, B.

{Nature Materials}, 10(3):189-193, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Potential explanation of charge response of magnetization in nanoporous systems

Subkow, S., Fähnle, M.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Herstellung und Qualifizierung gesputterter Magnesiumdiboridschichten

Breyer, F.

Hochschule Aalen, Aalen, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Large hidden orbital moments in magnetite

Goering, E.

{Physica Status Solidi B}, 248(10):2345-2351, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Cr magnetization reversal at the CrO2/RuO2 interface: Origin of the reduced GMR effect

Zafar, K., Audehm, P., Schütz, G., Goering, E., Pathak, M., Chetry, K. B., LeClair, P. R., Gupta, A.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetocaloric effect, magnetic domain structure and spin-reorientation transitios in HoCo5 single crystals

Skokov, K. P., Pastushenkov, Y. G., Koshkid\textquotesingleko, Y. S., Schütz, G., Goll, D., Ivanova, T. I., Nikitin, S. A., Semenova, E. M., Petrenko, A. V.

{Journal of Magnetism and Magnetic Materials}, 323(5):447-450, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Elucidating gating effects for hydrogen sorption in MFU-4-type triazolate-based metal-organic frameworks featuring different pore sizes

Denysenko, D., Grzywa, M., Tonigold, M., Streppel, B., Krkljus, I., Hirscher, M., Mugnaioli, E., Kolb, U., Hanss, J., Volkmer, D.

{Chemistry - A European Journal}, 17(6):1837-1848, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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BET specific surface area and pore structure of MOFs determined by hydrogen adsorption at 20 K

Streppel, B., Hirscher, M.

{Physical Chemistry Chemical Physics}, 13(8):3220-3222, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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High contrast magnetic and nonmagnetic sample current microscopy for bulk and transparent samples using soft X-rays

Nolle, D., Weigand, M., Schütz, G., Goering, E.

{Microscopy and Microanalysis}, 17, pages: 834-842, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic vortex core reversal by rotating magnetic fields generated on micrometer length scales

Curcic, M., Stoll, H., Weigand, M., Sackmann, V., Jüllig, P., Kammerer, M., Noske, M., Sproll, M., Van Waeyenberge, B., Vansteenkiste, A., Woltersdorf, G., Tyliszczak, T., Schütz, G.

{Physica Status Solidi B}, 248(10):2317-2322, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Operational Space Control of Constrained and Underactuated Systems

Mistry, M., Righetti, L.

In Proceedings of Robotics: Science and Systems, Los Angeles, CA, USA, June 2011 (inproceedings)

Abstract
The operational space formulation (Khatib, 1987), applied to rigid-body manipulators, describes how to decouple task-space and null-space dynamics, and write control equations that correspond only to forces at the end-effector or, alternatively, only to motion within the null-space. We would like to apply this useful theory to modern humanoids and other legged systems, for manipulation or similar tasks, however these systems present additional challenges due to their underactuated floating bases and contact states that can dynamically change. In recent work, Sentis et al. derived controllers for such systems by implementing a task Jacobian projected into a space consistent with the supporting constraints and underactuation (the so called "support consistent reduced Jacobian"). Here, we take a new approach to derive operational space controllers for constrained underactuated systems, by first considering the operational space dynamics within "projected inverse-dynamics" (Aghili, 2005), and subsequently resolving underactuation through the addition of dynamically consistent control torques. Doing so results in a simplified control solution compared with previous results, and importantly yields several new insights into the underlying problem of operational space control in constrained environments: 1) Underactuated systems, such as humanoid robots, cannot in general completely decouple task and null-space dynamics. However, 2) there may exist an infinite number of control solutions to realize desired task-space dynamics, and 3) these solutions involve the addition of dynamically consistent null-space motion or constraint forces (or combinations of both). In light of these findings, we present several possible control solutions, with varying optimization criteria, and highlight some of their practical consequences.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Formation of two amorphous phases in the Ni60Nb18Y22 alloy after high pressure torsion

Straumal, B. B., Mazilkin, A. A., Protasova, S. G., Goll, D., Baretzky, B., Bakai, A. S., Dobatkin, S. V.

{Kovove Materialy-Metallic Materials}, 49(1):17-22, 2011 (article)

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link (url) [BibTex]

link (url) [BibTex]