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2010


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Molecular QED of coherent and incoherent sum-frequency and second-harmonic generation in chiral liquids in the presence of a static electric field

Fischer, P., Salam, A.

MOLECULAR PHYSICS, 108(14):1857-1868, 2010 (article)

Abstract
Coherent second-order nonlinear optical processes are symmetry forbidden in centrosymmetric environments in the electric-dipole approximation. In liquids that contain chiral molecules, however, and which therefore lack mirror image symmetry, coherent sum-frequency generation is possible, whereas second-harmonic generation remains forbidden. Here we apply the theory of molecular quantum electrodynamics to the calculation of the matrix element, transition rate, and integrated signal intensity for sum-frequency and second-harmonic generation taking place in a chiral liquid in the presence and absence of a static electric field, to examine which coherent and incoherent processes exist in the electric-dipole approximation in liquids. Third- and fourth-order time-dependent perturbation theory is employed in combination with single-sided Feynman diagrams to evaluate two contributions arising from static field-free and field-induced processes. It is found that, in addition to the coherent term, an incoherent process exists for sum-frequency generation in liquids. Surprisingly, in the case of dc-field-induced second-harmonic generation, the incoherent contribution is found to always vanish for isotropic chiral liquids even though hyper-Rayleigh second-harmonic generation and electric-field-induced second-harmonic generation are both independently symmetry allowed in any liquid.

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DOI [BibTex]


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Dzyaloshinskii-Moriya interactions in systems with fabrication induced strain gradients: ab-initio study

Beck, P., Fähnle, M

{Journal of Magnetism and Magnetic Materials}, 322, pages: 3701-3703, 2010 (article)

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DOI [BibTex]


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On the nature of displacement bursts during nanoindentation of ultrathin Ni films on sapphire

Rabkin, E., Deuschle, J. K., Baretzky, B.

{Acta Materialia}, 58, pages: 1589-1598, 2010 (article)

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DOI [BibTex]


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Nanospheres generate out-of-plane magnetization

Amaladass, E., Ludescher, B., Schütz, G., Tyliszczak, T., Lee, M., Eimüller, T.

{Journal of Applied Physics}, 107, 2010 (article)

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DOI [BibTex]


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Temperature dependence of the magnetic properties of L10-FePt nanostructures and films

Bublat, T., Goll, D.

{Journal of Applied Physics}, 108(11), 2010 (article)

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DOI [BibTex]


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Magnetic properties of Fe nanoclusters on Cu(111) studied with X-ray magnetic circular dichroism

Fauth, K., Ballentine, G., Praetorius, C., Kleibert, A., Wilken, N., Voitkans, A., Meiwes-Broer, K.-H.

{Physica Status Solidi B}, 247(5):1170-1179, 2010 (article)

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DOI [BibTex]


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Nanoscale imaging using deep ultraviolet digital holographic microscopy

Faridian, A., Hopp, D., Pedrini, G., Eigenthaler, U., Hirscher, M., Osten, W.

{Optics Express}, 18(13):14159-14164, 2010 (article)

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DOI [BibTex]


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Metal-organic frameworks for hydrogen storage

Hirscher, M., Panella, B., Schmitz, B.

{Microporous and Mesoporous Materials}, 129, pages: 335-339, 2010 (article)

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DOI [BibTex]


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Samarium-cobalt 2:17 magnets: analysis of the coercive field of Sm2(CoFeCuZr)17 high-temperature permanent magnets

Goll, D., Stadelmaier, H. H., Kronmüller, H.

{Scripta Materialia}, 63, pages: 243-245, 2010 (article)

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DOI [BibTex]


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Low-temperature growth of silicon nanotubes and nanowires on amorphous substrates

Mbenkum, B. N., Schneider, A. S., Schütz, G., Xu, C., Richter, G., van Aken, P. A., Majer, G., Spatz, J. P.

{ACS Nano}, 4(4):1805-1812, 2010 (article)

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DOI [BibTex]


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Formation and mobility of protonic charge carriers in methyl sulfonic acid-water mixtures: A model for sulfonic acid based ionomers at low degree of hydration

Telfah, A., Majer, G., Kreuer, K. D., Schuster, M., Maier, J.

{Solid State Ionics}, 181, pages: 461-465, 2010 (article)

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Continuous photobleaching to study the growth modes of focal adhesions

de Beer, A. G. F., Majer, G., Roke, S., Spatz, J. P.

{Journal of Adhesion Science and Technology}, 24, pages: 2323-2334, 2010 (article)

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DOI [BibTex]


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Magnetic antivortex-core reversal by circular-rotational spin currents

Kamionka, T., Martens, M., Chou, K. W., Curcic, M., Drews, A., Schütz, G., Tyliszczak, T., Stoll, H., Van Waeyenberge, B., Meier, G.

{Physical Review Letters}, 105, 2010 (article)

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DOI [BibTex]


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Extension of Yafet\textquotesingles theory of spin relaxation to ferromagnets

Steiauf, D., Illg, C., Fähnle, M.

{Journal of Magnetism and Magnetic Materials}, 322, pages: L5-L7, 2010 (article)

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DOI [BibTex]


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Lateral transport of thermal capillary waves

Smith, T. H. R., Vasilyev, O., Maciolek, A., Schmidt, M.

{Europhysics Letters}, 89(1), 2010 (article)

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DOI [BibTex]


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The formation and propagation of flux avalanches in tailored MgB2 films

Treiber, S., Albrecht, J.

{New Journal of Physics}, 12, 2010 (article)

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DOI [BibTex]


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Direct imaging of current induced magnetic vortex gyration in an asymmetric potential well

Bisig, A., Rhensius, J., Kammerer, M., Curcic, M., Stoll, H., Schütz, G., Van Waeyenberge, B., Chou, K. W., Tyliszczak, T., Heyderman, L. J., Krzyk, S., von Bieren, A., Kläui, M.

{Applied Physics Letters}, 96, 2010 (article)

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DOI [BibTex]


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Induced magnetism of carbon atoms at the graphene/Ni(111) interface

Weser, M., Rehder, Y., Horn, K., Sicot, M., Fonin, M., Preobrajenski, A. B., Voloshina, E. N., Goering, E., Dedkov, Y. S.

{Applied Physics Letters}, 96, 2010 (article)

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DOI [BibTex]


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Photon counting system for time-resolved experiments in multibunch mode

Puzic, A., Korhonen, T., Kalantari, B., Raabe, J., Quitmann, C., Jüllig, P., Bommer, L., Goll, D., Schütz, G., Wintz, S., Strache, T., Körner, M., Markó, D., Bunce, C., Fassbender, J.

{Synchrotron Radiation News}, 23(2):26-32, 2010 (article)

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link (url) DOI [BibTex]


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Coupling of Fe and uncompensated Mn moments in exchange-biased Fe/MnPd

Brück, S., Macke, S., Goering, E., Ji, X., Zhan, Q., Krishnan, K. M.

{Physical Review B}, 81(13), 2010 (article)

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DOI [BibTex]


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Remarks about spillover and hydrogen adsorption - Comments on the contributions of A.V. Talyzin and R.T. Yang

Hirscher, M.

{Microporous and Mesoporous Materials}, 135, pages: 209-210, 2010 (article)

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Grain boundary ridges and triple lines

Straumal, B. B., Sursaeva, V. G., Baretzky, B.

{Scripta Materialia}, 62(12):924-927, 2010 (article)

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DOI [BibTex]


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Expanding micelle nanolithography to the self-assembly of multicomponent core-shell nanoparticles

Mbenkum, B. N., D\’\iaz-Ortiz, A., Gu, L., van Aken, P. A., Schütz, G.

{Journal of the American Chemical Society}, 132(31):10671-10673, 2010 (article)

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Hydrogen spillover measurements of unbridged and bridged metal-organic frameworks - revisited

Campesi, R., Cuevas, F., Latroche, M., Hirscher, M.

{Physical Chemistry Chemical Physics}, 12, pages: 10457-10459, 2010 (article)

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Relating Gilbert damping and ultrafast laser-induced demagnetization

Fähnle, M., Seib, J., Illg, C.

{Physical Review B}, 82, 2010 (article)

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Ferromagnetic properties of the Mn-doped nanograined ZnO films

Straumal, B. B., Protasova, S. G., Mazilkin, A. A., Myatiev, A. A., Straumal, P. B., Schütz, G., Goering, E., Baretzky, B.

{Journal of Applied Physics}, 108, 2010 (article)

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Ubiquity of ferromagnetic signals in common diamagnetic oxide crystals

Khalid, M., Setzer, A., Ziese, M., Esquinazi, P., Spemann, D., Pöppl, A., Goering, E.

{Physical Review B}, 81(21), 2010 (article)

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Calculation of the Gilbert damping matrix at low scattering rates in Gd

Seib, J., Fähnle, M.

{Physical Review B}, 82, 2010 (article)

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DOI [BibTex]


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Swift heavy ions for controlled modification of soft magnetic properties of Fe0.85N0.15 thin film

Gupta, R., Gupta, A., Bhatt, R., Rüffer, R., Avasthi, D. K.

{Journal of Physics: Condensed Matter}, 22(22), 2010 (article)

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DOI [BibTex]


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Laterally driven interfaces in the three-dimensional Ising lattice gas

Smith, T. H. R., Vasilyev, O., Maciolek, A., Schmidt, M.

{Physical Review E}, 82(2), 2010 (article)

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DOI [BibTex]


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Samarium-cobalt 2:17 magnets: identifying Smn+1Co5n-1 phases stabilized by Zr

Stadelmaier, H. H., Kronmüller, H., Goll, D.

{Scripta Materialia}, 63, pages: 843-846, 2010 (article)

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DOI [BibTex]

DOI [BibTex]


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Planar metamaterial analogue of electromagnetically induced transparancy for plasmonic sensing

Liu, N., Weiss, T., Mesch, M., Langguth, L., Eigenthaler, U., Hirscher, M., Sönnichsen, C., Giessen, H.

{Nano Letters}, 10, pages: 1103-1107, 2010 (article)

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DOI [BibTex]


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Explaining the paradoxical diversity of ultrafast last-induced demagnetization

Koopmans, B., Malinowski, G., Dalla Longa, F., Steiauf, D., Fähnle, M., Roth, T., Cinchetti, M., Aeschlimann, M.

{Nature Materials}, 9, pages: 259-265, 2010 (article)

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DOI [BibTex]


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A high heat of adsorption for hydrogen in magnesium formate

Schmitz, B., Krkljus, I., Leung, E., Höffken, H. W., Müller, U., Hirscher, M.

{ChemSusChem}, 3, pages: 758-761, 2010 (article)

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Force induced destabilization of adhesion complexes at defined integrin spacings on nanostructured surfaces

de Beer, A. G. F., Cavalcanti-Adam, E. A., Majer, G., López-Garc\’\ia, M., Kessler, H., Spatz, J. P.

{Physical Review E}, 81, 2010 (article)

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Anisotropic damping of the magnetization dynamics in Ni, Co, and Fe

Gilmore, K., Stiles, M. D., Seib, J., Steiauf, D., Fähnle, M.

{Physical Review B}, 81, 2010 (article)

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Influence of [Mo6Br8F6]2- cluster inclusion within the mesoporous solid MIL-101 on hydrogen storage performance

Dybtsev, D., Serre, C., Schmitz, B., Panella, B., Hirscher, M., Latroche, M., Llewellyn, P. L., Cordier, S., Molard, Y., Haouas, M., Taulelle, F., Férey, G.

{Langmuir}, 26(13):11283-11290, 2010 (article)

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Grain boundary layers in nanocrystalline ferromagnetic zinc oxide

Straumal, B. B., Myatiev, A. A., Straumal, P. B., Mazilkin, A. A., Protasova, S. G., Goering, E., Baretzky, B.

{JETP Letters}, 92(6):396-400, 2010 (article)

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2006


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Chiral molecules split light: Reflection and refraction in a chiral liquid

Ghosh, A., Fischer, P.

PHYSICAL REVIEW LETTERS, 97(17), 2006, Featured highlight ‘Fundamental optical physics: Refraction’ Nature Photonics, Nov. 2006. (article)

Abstract
A light beam changes direction as it enters a liquid at an angle from another medium, such as air. Should the liquid contain molecules that lack mirror symmetry, then it has been predicted by Fresnel that the light beam will not only change direction, but will actually split into two separate beams with a small difference in the respective angles of refraction. Here we report the observation of this phenomenon. We also demonstrate that the angle of reflection does not equal the angle of incidence in a chiral medium. Unlike conventional optical rotation, which depends on the path-length through the sample, the reported reflection and refraction phenomena arise within a few wavelengths at the interface and thereby suggest a new approach to polarimetry that can be used in microfluidic volumes.

Featured highlight ‘Fundamental optical physics: Refraction’ Nature Photonics, Nov. 2006.

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Direct chiral discrimination in NMR spectroscopy

Buckingham, A., Fischer, P.

CHEMICAL PHYSICS, 324(1):111-116, 2006 (article)

Abstract
Conventional nuclear magnetic resonance spectroscopy is unable to distinguish between the two mirror-image forms (enantiomers) of a chiral molecule. This is because the NMR spectrum is determined by the chemical shifts and spin-spin coupling constants which - in the absence of a chiral solvent - are identical for the two enantiomers. We discuss how chirality may nevertheless be directly detected in liquid-state NMR spectroscopy: In a chiral molecule, the rotating nuclear magnetic moment induces an electric dipole moment in the direction perpendicular to itself and to the permanent magnetic field of the spectrometer. We present computations of the precessing electric polarization following a pi/2 pulse. Our estimates indicate that the electric polarization should be detectable in favourable cases. We also predict that application of an electrostatic field induces a chirally sensitive magnetization oscillating in the direction of the permanent magnetic field. We show that the electric-field-perturbed chemical shift tensor, the nuclear magnetic shielding polarizability, underlies these chiral NMR effects. (c) 2005 Elsevier B.V. All rights reserved.

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Ring-resonator-based frequency-domain optical activity measurements of a chiral liquid

Vollmer, F., Fischer, P.

OPTICS LETTERS, 31(4):453-455, 2006 (article)

Abstract
Chiral liquids rotate the plane of polarization of linearly polarized light and are therefore optically active. Here we show that optical rotation can be observed in the frequency domain. A chiral liquid introduced in a fiber-loop ring resonator that supports left and right circularly polarized modes gives rise to relative frequency shifts that are a direct measure of the liquid's circular birefringence and hence of its optical activity. The effect is in principle not diminished if the circumference of the ring is reduced. The technique is similarly applicable to refractive index and linear birefringence measurements. (c) 2006 Optical Society of America.

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Sign of the refractive index in a gain medium with negative permittivity and permeability

Chen, Y., Fischer, P., Wise, F.

JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 23(1):45-50, 2006 (article)

Abstract
We show how the sign of the refractive index in any medium may be derived using a rigorous analysis based on Einstein causality. In particular, we consider left-handed materials, i.e., media that have negative permittivities and permeabilities at the frequency of interest. We find that the consideration of gain in such media can give rise to a positive refractive index. (c) 2006 Optical Society of America.

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DOI [BibTex]


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Influence of the substrate on the magnetic anisotropy of monatomic wires

Komelj, M., Steiauf, D., Fähnle, M.

{Physical Review B}, 73, 2006 (article)

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Mechanical properties of single-walled carbon nanotubes based on higher order Cauchy-Born rule

Guo, X., Wang, J. B., Zhang, H. W.

{International Journal of Solids and Structures}, 43, pages: 1276-1290, 2006 (article)

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Vanishing Fe 3d orbital moments in single-crystalline magnetite

Goering, E., Gold, S., Lafkioti, M., Schütz, G.

{Europhysics Letters}, 73(1):97-103, 2006 (article)

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Enhancement of L10 phase formation in FePt nanoparticles by nitrogenization

Dmitrieva, O., Acet, M., Dumpich, G., Kästner, J., Antoniak, C., Farle, M., Fauth, K.

{Journal of Physics D}, 39, pages: 4741-4745, 2006 (article)

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Structure of historical brass tonques and shallots from baroque organs

Baretzky, B., Friesel, M., Petelin, A., Mazilkin, A., Straumal, B.

{Defect and Diffusion Forum}, 249, pages: 275-280, 2006 (article)

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Three-dimensional modeling of mechanical forces in the extra-cellular matrix during epithelial lumen formation

Zeng, D., Ferrari, A., Ulmer, J., Veligodskiy, A., Fischer, P., Spatz, J. P., Ventikos, Y., Poulikakos, D., Kroschewski, R.

{Biophysical Journal}, 90(12):4380-4391, 2006 (article)

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