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Effect of the soft layer thickness of magnetization reversal process of exchange-spring nanomagnet patterns

Son, K., Schütz, G., Goering, E.

{Current Applied Physics}, 20(4):477-483, Elsevier B.V., Amsterdam, 2020 (article)

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DOI [BibTex]


{Creating zero-field skyrmions in exchange-biased multilayers through X-ray illumination}
Creating zero-field skyrmions in exchange-biased multilayers through X-ray illumination

Guang, Y., Bykova, I., Liu, Y., Yu, G., Goering, E., Weigand, M., Gräfe, J., Kim, S. K., Zhang, J., Zhang, H., Yan, Z., Wan, C., Feng, J., Wang, X., Guo, C., Wei, H., Peng, Y., Tserkovnyak, Y., Han, X., Schütz, G.

{Nature Communications}, 11, Nature Publishing Group, London, 2020 (article)

Abstract
Skyrmions, magnetic textures with topological stability, hold promises for high-density and energy-efficient information storage devices owing to their small size and low driving-current density. Precise creation of a single nanoscale skyrmion is a prerequisite to further understand the skyrmion physics and tailor skyrmion-based applications. Here, we demonstrate the creation of individual skyrmions at zero-field in an exchange-biased magnetic multilayer with exposure to soft X-rays. In particular, a single skyrmion with 100-nm size can be created at the desired position using a focused X-ray spot of sub-50-nm size. This single skyrmion creation is driven by the X-ray-induced modification of the antiferromagnetic order and the corresponding exchange bias. Furthermore, artificial skyrmion lattices with various arrangements can be patterned using X-ray. These results demonstrate the potential of accurate optical control of single skyrmion at sub-100 nm scale. We envision that X-ray could serve as a versatile tool for local manipulation of magnetic orders.

mms

DOI [BibTex]

DOI [BibTex]


{Tuning the magnetic properties of permalloy-based magnetoplasmonic crystals for sensor applications}
Tuning the magnetic properties of permalloy-based magnetoplasmonic crystals for sensor applications

Murzin, D. V., Belyaev, V. K., Groß, F., Gräfe, J., Rivas, M., Rodionova, V. V.

{Japanese Journal of Applied Physics}, 59(SE), IOP Publishing Ltd, Bristol, England, 2020 (article)

Abstract
Miniature magnetic sensors based on magnetoplasmonic crystals (MPlCs) exhibit high sensitivity and high spatial resolution, which can be obtained by the excitation of surface plasmon polaritons. A field dependence of surface plasmon polaritons' enhanced magneto-optical response strongly correlates with magnetic properties of MPlCs that can be tuned by changing spatial parameters, such as the period and height of diffraction gratings and thicknesses of functional layers. This work compares the magnetic properties of MPlCs based on Ni80Fe20 (permalloy) obtained from local (longitudinal magneto-optical Kerr effect) and bulk (vibrating-sample magnetometry) measurements and demonstrates an ability to control sensors' performance through changing the magnetic properties of the MPlCs. The influence of the substrate's geometry (planar or sinusoidal and trapezoidal diffraction grating profiles) and the thickness of the surface layer is examined.

mms

DOI [BibTex]

DOI [BibTex]


Excursion Search for Constrained Bayesian Optimization under a Limited Budget of Failures
Excursion Search for Constrained Bayesian Optimization under a Limited Budget of Failures

Marco, A., Rohr, A. V., Baumann, D., Hernández-Lobato, J. M., Trimpe, S.

2020 (proceedings) In revision

Abstract
When learning to ride a bike, a child falls down a number of times before achieving the first success. As falling down usually has only mild consequences, it can be seen as a tolerable failure in exchange for a faster learning process, as it provides rich information about an undesired behavior. In the context of Bayesian optimization under unknown constraints (BOC), typical strategies for safe learning explore conservatively and avoid failures by all means. On the other side of the spectrum, non conservative BOC algorithms that allow failing may fail an unbounded number of times before reaching the optimum. In this work, we propose a novel decision maker grounded in control theory that controls the amount of risk we allow in the search as a function of a given budget of failures. Empirical validation shows that our algorithm uses the failures budget more efficiently in a variety of optimization experiments, and generally achieves lower regret, than state-of-the-art methods. In addition, we propose an original algorithm for unconstrained Bayesian optimization inspired by the notion of excursion sets in stochastic processes, upon which the failures-aware algorithm is built.

ics am

arXiv code (python) PDF [BibTex]


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Analytical classical density functionals from an equation learning network

Lin, S., Martius, G., Oettel, M.

The Journal of Chemical Physics, 152(2):021102, 2020, arXiv preprint \url{https://arxiv.org/abs/1910.12752} (article)

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Preprint_PDF DOI [BibTex]

Preprint_PDF DOI [BibTex]


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Element-resolved study of the evolution of magnetic response in FexN compounds

Chen, Y., Gölden, D., Dirba, I., Huang, M., Gutfleisch, O., Nagel, P., Merz, M., Schuppler, S., Schütz, G., Alff, L., Goering, E.

{Journal of Magnetism and Magnetic Materials}, 498, NH, Elsevier, Amsterdam, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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The role of temperature and drive current in skyrmion dynamics

Litzius, K., Leliaert, J., Bassirian, P., Rodrigues, D., Kromin, S., Lemesh, I., Zazvorka, J., Lee, K., Mulkers, J., Kerber, N., Heinze, D., Keil, N., Reeve, R. M., Weigand, M., Van Waeyenberge, B., Schütz, G., Everschor-Sitte, K., Beach, G. S. D., Kläui, M.

{Nature Electronics}, 3(1):30-36, Springer Nature, London, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic flux penetration into micron-sized superconductor/ferromagnet bilayers

Simmendinger, J., Weigand, M., Schütz, G., Albrecht, J.

{Superconductor Science and Technology}, 33(2), IOP Pub., Bristol, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Fabrication and temperature-dependent magnetic properties of large-area L10-FePt/Co exchange-spring magnet nanopatterns

Son, K., Schütz, G.

{Physica E: Low-Dimensional Systems And Nanostructures}, 115, North-Holland, Amsterdam, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


Magnetic Anisotropy in Thin Layers of (Mn,Zn)Fe2O4 on SrTiO3 (001)
Magnetic Anisotropy in Thin Layers of (Mn,Zn)Fe2O4 on SrTiO3 (001)

Denecke, R., Welke, M., Huth, P., Gräfe, J., Brachwitz, K., Lorenz, M., Grundmann, M., Ziese, M., Esquinazi, P. D., Goering, E., Schütz, G., Schindler, K., Chassé, A.

physica status solidi (b), n/a(n/a):1900627, 2020 (article)

Abstract
Herein, a ferrimagnetic manganese zinc ferrite (Mn0.5Zn0.5Fe2O4) film with a thickness of 200 nm is prepared without a buffer layer on strontium titanate (001) (SrTiO3) using pulsed laser deposition. Its magnetic properties are investigated using superconducting quantum interference device (SQUID), X-ray absorption spectroscopy with subsequent X-ray magnetic circular dichroism (XMCD) and magneto-optic Kerr effect (MOKE). Hysteresis loops derived from SQUID exhibits bulk-like properties. This can further be confirmed by bulk-like XMCD spectra. In remanent magnetization, an in-plane magnetization with basically no out-of-plane component is found. The magnetic moments derived by the sum rule formalism from the XMCD data are in good agreement to the magnetization observed by SQUID and MOKE. XMCD as well as MOKE reveal an in-plane angular fourfold magnetic anisotropy with the easy direction along [110] for (Mn0.5Zn0.5)Fe2O4 on SrTiO3. The element-specific magnetic moments from XMCD show a stronger contribution of Fe to the anisotropy than of Mn and distinct contributions of the orbital moments.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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How to functionalise metal-organic frameworks to enable guest nanocluster embedment

King, J., Zhang, L., Doszczeczko, S., Sambalova, O., Luo, H., Rohman, F., Phillips, O., Borgschulte, A., Hirscher, M., Addicoat, M., Szilágyi, P. A.

{Journal of Materials Chemistry A}, 8(9):4889-4897, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic and microstructural properties of anisotropic MnBi magnets compacted by spark plasma sintering

Chen, Y., Gregori, G., Rheingans, B., Huang, W., Kronmüller, H., Schütz, G., Goering, E.

{Journal of Alloys and Compounds}, 830, Elsevier B.V., Lausanne, Switzerland, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


Safe and Fast Tracking on a Robot Manipulator: Robust MPC and Neural Network Control
Safe and Fast Tracking on a Robot Manipulator: Robust MPC and Neural Network Control

Nubert, J., Koehler, J., Berenz, V., Allgower, F., Trimpe, S.

IEEE Robotics and Automation Letters, 2020 (article) Accepted

Abstract
Fast feedback control and safety guarantees are essential in modern robotics. We present an approach that achieves both by combining novel robust model predictive control (MPC) with function approximation via (deep) neural networks (NNs). The result is a new approach for complex tasks with nonlinear, uncertain, and constrained dynamics as are common in robotics. Specifically, we leverage recent results in MPC research to propose a new robust setpoint tracking MPC algorithm, which achieves reliable and safe tracking of a dynamic setpoint while guaranteeing stability and constraint satisfaction. The presented robust MPC scheme constitutes a one-layer approach that unifies the often separated planning and control layers, by directly computing the control command based on a reference and possibly obstacle positions. As a separate contribution, we show how the computation time of the MPC can be drastically reduced by approximating the MPC law with a NN controller. The NN is trained and validated from offline samples of the MPC, yielding statistical guarantees, and used in lieu thereof at run time. Our experiments on a state-of-the-art robot manipulator are the first to show that both the proposed robust and approximate MPC schemes scale to real-world robotic systems.

am ics

arXiv PDF DOI [BibTex]

arXiv PDF DOI [BibTex]


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Generation and characterization of focused helical x-ray beams

Loetgering, L., Baluktsian, M., Keskinbora, K., Horstmeyer, R., Wilhein, T., Schütz, G., Eikema, K. S. E., Witte, S.

Science Advances, 6(7), American Association for the Advancement of Science, 2020 (article)

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Generation and characterization of focused helical x-ray beams link (url) DOI [BibTex]

Generation and characterization of focused helical x-ray beams link (url) DOI [BibTex]


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Materials for hydrogen-based energy storage - past, recent progress and future outlook

Hirscher, M., Yartys, V. A., Baricco, M., Bellosta von Colbe, J., Blanchard, D., Bowman Jr., R. C., Broom, D. P., Buckley, C. E., Chang, F., Chen, P., Cho, Y. W., Crivello, J., Cuevas, F., David, W. I. F., de Jongh, P. E., Denys, R. V., Dornheim, M., Felderhoff, M., Filinchuk, Y., Froudakis, G. E., Grant, D. M., Gray, E. M., Hauback, B. C., He, T., Humphries, T. D., Jensen, T. R., Kim, S., Kojima, Y., Latroche, M., Li, H., Lotostskyy, M. V., Makepeace, J. W., M\oller, K. T., Naheed, L., Ngene, P., Noréus, D., Nyg\aard, M. M., Orimo, S., Paskevicius, M., Pasquini, L., Ravnsbaek, D. B., Sofianos, M. V., Udovic, T. J., Vegge, T., Walker, G. S., Webb, C. J., Weidenthaler, C., Zlotea, C.

{Journal of Alloys and Compounds}, 827, Elsevier B.V., Lausanne, Switzerland, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


{Thermal nucleation and high-resolution imaging of submicrometer magnetic bubbles in thin thulium iron garnet films with perpendicular anisotropy}
Thermal nucleation and high-resolution imaging of submicrometer magnetic bubbles in thin thulium iron garnet films with perpendicular anisotropy

Büttner, F., Mawass, M. A., Bauer, J., Rosenberg, E., Caretta, L., Avci, C. O., Gräfe, J., Finizio, S., Vaz, C. A. F., Novakovic, N., Weigand, M., Litzius, K., Förster, J., Träger, N., Groß, F., Suzuki, D., Huang, M., Bartell, J., Kronast, F., Raabe, J., Schütz, G., Ross, C. A., Beach, G. S. D.

{Physical Review Materials}, 4(1), American Physical Society, College Park, MD, 2020 (article)

Abstract
Ferrimagnetic iron garnets are promising materials for spintronics applications, characterized by ultralow damping and zero current shunting. It has recently been found that few nm-thick garnet films interfaced with a heavy metal can also exhibit sizable interfacial spin-orbit interactions, leading to the emergence, and efficient electrical control, of one-dimensional chiral domain walls. Two-dimensional bubbles, by contrast, have so far only been confirmed in micrometer-thick films. Here, we show by high resolution scanning transmission x-ray microscopy and photoemission electron microscopy that submicrometer bubbles can be nucleated and stabilized in ∼25-nm-thick thulium iron garnet films via short heat pulses generated by electric current in an adjacent Pt strip, or by ultrafast laser illumination. We also find that quasistatic processes do not lead to the formation of a bubble state, suggesting that the thermodynamic path to reaching that state requires transient dynamics. X-ray imaging reveals that the bubbles have Bloch-type walls with random chirality and topology, indicating negligible chiral interactions at the garnet film thickness studied here. The robustness of thermal nucleation and the feasibility demonstrated here to image garnet-based devices by x-rays both in transmission geometry and with sensitivity to the domain wall chirality are critical steps to enabling the study of small spin textures and dynamics in perpendicularly magnetized thin-film garnets.

mms

DOI [BibTex]

DOI [BibTex]


{Real-space imaging of confined magnetic skyrmion tubes}
Real-space imaging of confined magnetic skyrmion tubes

Birch, M. T., Cortés-Ortuño, D., Turnbull, L. A., Wilson, M. N., Groß, F., Träger, N., Laurenson, A., Bukin, N., Moody, S. H., Weigand, M., Schütz, G., Popescu, H., Fan, R., Steadman, P., Verezhak, J. A. T., Balakrishnan, G., Loudon, J. C., Twitchett-Harrison, A. C., Hovorka, O., Fangohr, H., Ogrin, F., Gräfe, J., Hatton, P. D.

Nature Communications, 11, pages: 1726, 2020 (article)

Abstract
Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the host material. The study of this skyrmion tube state (SkT) is vital for furthering the understanding of skyrmion formation and dynamics for future applications. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we demonstrate the real-space observation of skyrmion tubes in a lamella of FeGe using resonant magnetic x-ray imaging and comparative micromagnetic simulations, confirming their extended structure. The formation of these structures at the edge of the sample highlights the importance of confinement and edge effects in the stabilisation of the SkT state, opening the door to further investigation into this unexplored dimension of the skyrmion spin texture.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Room temperature ferromagnetism driven by Ca-doped BiFeO3 multiferroic functional material

Marzouk, M., Hashem, H. M., Soltan, S., Ramadan, A. A.

{Journal of Materials Science: Materials in Electronics}, 31(7):5599-5607, Springer, Norwell, MA, 2020 (article)

mms

DOI [BibTex]

DOI [BibTex]

1997


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Locally weighted learning

Atkeson, C. G., Moore, A. W., Schaal, S.

Artificial Intelligence Review, 11(1-5):11-73, 1997, clmc (article)

Abstract
This paper surveys locally weighted learning, a form of lazy learning and memory-based learning, and focuses on locally weighted linear regression. The survey discusses distance functions, smoothing parameters, weighting functions, local model structures, regularization of the estimates and bias, assessing predictions, handling noisy data and outliers, improving the quality of predictions by tuning fit parameters, interference between old and new data, implementing locally weighted learning efficiently, and applications of locally weighted learning. A companion paper surveys how locally weighted learning can be used in robot learning and control. Keywords: locally weighted regression, LOESS, LWR, lazy learning, memory-based learning, least commitment learning, distance functions, smoothing parameters, weighting functions, global tuning, local tuning, interference.

am

link (url) [BibTex]

1997


link (url) [BibTex]


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Locally weighted learning for control

Atkeson, C. G., Moore, A. W., Schaal, S.

Artificial Intelligence Review, 11(1-5):75-113, 1997, clmc (article)

Abstract
Lazy learning methods provide useful representations and training algorithms for learning about complex phenomena during autonomous adaptive control of complex systems. This paper surveys ways in which locally weighted learning, a type of lazy learning, has been applied by us to control tasks. We explain various forms that control tasks can take, and how this affects the choice of learning paradigm. The discussion section explores the interesting impact that explicitly remembering all previous experiences has on the problem of learning to control. Keywords: locally weighted regression, LOESS, LWR, lazy learning, memory-based learning, least commitment learning, forward models, inverse models, linear quadratic regulation (LQR), shifting setpoint algorithm, dynamic programming.

am

link (url) [BibTex]

link (url) [BibTex]

1995


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Memory-based neural networks for robot learning

Atkeson, C. G., Schaal, S.

Neurocomputing, 9, pages: 1-27, 1995, clmc (article)

Abstract
This paper explores a memory-based approach to robot learning, using memory-based neural networks to learn models of the task to be performed. Steinbuch and Taylor presented neural network designs to explicitly store training data and do nearest neighbor lookup in the early 1960s. In this paper their nearest neighbor network is augmented with a local model network, which fits a local model to a set of nearest neighbors. This network design is equivalent to a statistical approach known as locally weighted regression, in which a local model is formed to answer each query, using a weighted regression in which nearby points (similar experiences) are weighted more than distant points (less relevant experiences). We illustrate this approach by describing how it has been used to enable a robot to learn a difficult juggling task. Keywords: memory-based, robot learning, locally weighted regression, nearest neighbor, local models.

am

link (url) [BibTex]

1995


link (url) [BibTex]

1993


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Design concurrent calculation: A CAD- and data-integrated approach

Schaal, S., Ehrlenspiel, K.

Journal of Engineering Design, 4, pages: 71-85, 1993, clmc (article)

Abstract
Besides functional regards, product design demands increasingly more for further reaching considerations. Quality alone cannot suffice anymore to compete in the market; design for manufacturability, for assembly, for recycling, etc., are well-known keywords. Those can largely be reduced to the necessity of design for costs. This paper focuses on a CAD-based approach to design concurrent calculation. It will discuss how, in the meantime well-established, tools like feature technology, knowledge-based systems, and relational databases can be blended into one coherent concept to achieve an entirely CAD- and data-integrated cost information tool. This system is able to extract data from the CAD-system, combine it with data about the company specific manufacturing environment, and subsequently autonomously evaluate manufacturability aspects and costs of the given CAD-model. Within minutes the designer gets quantitative in-formation about the major cost sources of his/her design. Additionally, some alternative methods for approximating manu-facturing times from empirical data, namely neural networks and local weighted regression, are introduced.

am

[BibTex]

1993


[BibTex]


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textes
(article)

mms

[BibTex]


[BibTex]