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2020


Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles
Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles

Singh, D., Domínguez, A., Choudhury, U., Kottapalli, S., Popescu, M., Dietrich, S., Fischer, P.

Nature Communications, 11(2210), May 2020 (article)

Abstract
Symmetry breaking and the emergence of self-organized patterns is the hallmark of com- plexity. Here, we demonstrate that a sessile drop, containing titania powder particles with negligible self-propulsion, exhibits a transition to collective motion leading to self-organized flow patterns. This phenomenology emerges through a novel mechanism involving the interplay between the chemical activity of the photocatalytic particles, which induces Mar- angoni stresses at the liquid–liquid interface, and the geometrical confinement provided by the drop. The response of the interface to the chemical activity of the particles is the source of a significantly amplified hydrodynamic flow within the drop, which moves the particles. Furthermore, in ensembles of such active drops long-ranged ordering of the flow patterns within the drops is observed. We show that the ordering is dictated by a chemical com- munication between drops, i.e., an alignment of the flow patterns is induced by the gradients of the chemicals emanating from the active particles, rather than by hydrodynamic interactions.

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Axisymmetric spheroidal squirmers and self-diffusiophoretic particles

Pöhnl, R., Popescu, M. N., Uspal, W. E.

Journal of Physics: Condensed Matter, 32(16), IOP Publishing, Bristol, 2020 (article)

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Tracer diffusion on a crowded random Manhattan lattice

Mej\’\ia-Monasterio, C., Nechaev, S., Oshanin, G., Vasilyev, O.

New Journal of Physics, 22(3), IOP Publishing, Bristol, 2020 (article)

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Wetting transitions on soft substrates

Napiorkowski, M., Schimmele, L., Dietrich, S.

{EPL}, 129(1), EDP Science, Les-Ulis, 2020 (article)

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Blessing and Curse: How a Supercapacitor Large Capacitance Causes its Slow Charging

Lian, C., Janssen, M., Liu, H., van Roij, R.

Physical Review Letters, 124(7), American Physical Society, Woodbury, N.Y., 2020 (article)

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Interplay of quenching temperature and drift in Brownian dynamics

Khalilian, H., Nejad, M. R., Moghaddam, A. G., Rohwer, C. M.

EPL, 128(6), EDP Science, Les-Ulis, 2020 (article)

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Fractal-seaweeds type functionalization of graphene

Amsharov, K., Sharapa, D. I., Vasilyev, O. A., Martin, O., Hauke, F., Görling, A., Soni, H., Hirsch, A.

Carbon, 158, pages: 435-448, Elsevier, Amsterdam, 2020 (article)

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Effective pair interaction of patchy particles in critical fluids

Farahmand Bafi, N., Nowakowski, P., Dietrich, S.

The Journal of Chemical Physics, 152(11), American Institute of Physics, Woodbury, N.Y., 2020 (article)

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Cassie-Wenzel transition of a binary liquid mixture on a nanosculptured surface

Singh, S. L., Schimmele, L., Dietrich, S.

Physical Review E, 101(5), American Physical Society, Melville, NY, 2020 (article)

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Energy storage in steady states under cyclic local energy input

Zhang, Y., Holyst, R., Maciolek, A.

Physical Review E, 101(1), American Physical Society, Melville, NY, 2020 (article)

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Numerical simulations of self-diffusiophoretic colloids at fluid interfaces

Peter, T., Malgaretti, P., Rivas, N., Scagliarini, A., Harting, J., Dietrich, S.

Soft Matter, 16(14):3536-3547, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

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2019


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Dynamics of beneficial epidemics

Berdahl, A., Brelsford, C., De Bacco, C., Dumas, M., Ferdinand, V., Grochow, J. A., nt Hébert-Dufresne, L., Kallus, Y., Kempes, C. P., Kolchinsky, A., Larremore, D. B., Libby, E., Power, E. A., A., S. C., Tracey, B. D.

Scientific Reports, 9, pages: 15093, October 2019 (article)

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2019


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Response of active Brownian particles to shear flow

Asheichyk, K., Solon, A., Rohwer, C. M., Krüger, M.

The Journal of Chemical Physics, 150(14), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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Vortex Mass in the Three-Dimensional O(2) Scalar Theory

Delfino, G., Selke, W., Squarcini, A.

Physical Review Letters, 122(5), American Physical Society, Woodbury, N.Y., 2019 (article)

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Dynamics near planar walls for various model self-phoretic particles

Bayati, P., Popescu, M. N., Uspal, W. E., Dietrich, S., Najafi, A.

Soft Matter, 15(28):5644-5672, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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Glucose Oxidase Micropumps: Multi-Faceted Effects of Chemical Activity on Tracer Particles Near the Solid-Liquid Interface

Munteanu, R. E., Popescu, M. N., Gáspár, S.

Condensed Matter, 4(3), MDPI, Basel, 2019 (article)

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Criticality senses topology

Vasilyev, O. A., Maciolek, A., Dietrich, S.

EPL, 128(2), EDP Science, Les-Ulis, 2019 (article)

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Drag Force for Asymmetrically Grafted Colloids in Polymer Solutions

Werner, M., Malgaretti, P., Maciolek, A.

Frontiers in Physics, 7, Frontiers Media, Lausanne, 2019 (article)

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Feeling Your Neighbors across the Walls: How Interpore Ionic Interactions Affect Capacitive Energy Storage

Kondrat, S., Vasilyev, O., Kornyshev, A. A.

The Journal of Physical Chemistry Letters, 10(16):4523-4527, American Chemical Society, Washington, DC, 2019 (article)

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Active Janus colloids at chemically structured surfaces

Uspal, W. E., Popescu, M. N., Dietrich, S., Tasinkevych, M.

The Journal of Chemical Physics, 150(20), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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Illumination-induced motion of a Janus nanoparticle in binary solvents

Araki, T., Maciolek, A.

Soft Matter, 15(26):5243-5254, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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Transient response of an electrolyte to a thermal quench

Janssen, M., Bier, M.

Physical Review E, 99(4), American Physical Society, Melville, NY, 2019 (article)

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Aging phenomena during phase separation in fluids: decay of autocorrelation for vapor\textendashliquid transitions

Roy, Sutapa, Bera, Arabinda, Majumder, Suman, Das, Subir K.

Soft Matter, 15(23):4743-4750, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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Flux and storage of energy in nonequilibrium stationary states

Holyst, R., Maciolek, A., Zhang, Y., Litniewski, M., Knycha\la, P., Kasprzak, M., Banaszak, M.

Physical Review E, 99(4), American Physical Society, Melville, NY, 2019 (article)

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Correlations and forces in sheared fluids with or without quenching

Rohwer, C. M., Maciolek, A., Dietrich, S., Krüger, M.

New Journal of Physics, 21, IOP Publishing, Bristol, 2019 (article)

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Ensemble dependence of critical Casimir forces in films with Dirichlet boundary conditions

Rohwer, C. M., Squarcini, A., Vasilyev, O., Dietrich, S., Gross, M.

Physical Review E, 99(6), American Physical Society, Melville, NY, 2019 (article)

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Controlling the dynamics of colloidal particles by critical Casimir forces

Magazzù, A., Callegari, A., Staforelli, J. P., Gambassi, A., Dietrich, S., Volpe, G.

Soft Matter, 15(10):2152-2162, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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Charge regulation radically modifies electrostatics in membrane stacks

Majee, A., Bier, M., Blossey, R., Podgornik, R.

Physical Review E, 100(5), American Physical Society, Melville, NY, 2019 (article)

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Comment on "Which interactions dominate in active colloids?" [J. Chem. Phys. 150, 061102 (2019)]

Popescu, M. N., Dominguez, A., Uspal, W. E., Tasinkevych, M., Dietrich, S.

The Journal of Chemical Physics, 151(6), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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Current-mediated synchronization of a pair of beating non-identical flagella

Dotsenko, V., Maciolek, A., Oshanin, G., Vasilyev, O., Dietrich, S.

New Journal of Physics, 21, IOP Publishing, Bristol, 2019 (article)

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Driving an electrolyte through a corrugated nanopore

Malgaretti, P., Janssen, M., Pagonabarraga, I., Rubi, J. M.

The Journal of Chemical Physics, 151(8), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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Spectral Content of a Single Non-Brownian Trajectory

Krapf, D., Lukat, N., Marinari, E., Metzler, R., Oshanin, G., Selhuber-Unkel, C., Squarcini, A., Stadler, L., Weiss, M., Xu, X.

Physical Review X, 9(1), American Physical Society, New York, NY, 2019 (article)

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Curvature affects electrolyte relaxation: Studies of spherical and cylindrical electrodes

Janssen, M.

Physical Review E, 100(4), American Physical Society, Melville, NY, 2019 (article)

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Dynamics of the critical Casimir force for a conserved order parameter after a critical quench

Gross, M., Rohwer, C. M., Dietrich, S.

Physical Review E, 100(1), American Physical Society, Melville, NY, 2019 (article)

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Interface structures in ionic liquid crystals

Bartsch, H., Bier, M., Dietrich, S.

Soft Matter, 15(20):4109-4126, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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Interfacial premelting of ice in nano composite materials

Li, H., Bier, M., Mars, J., Weiss, H., Dippel, A., Gutowski, O., Honkimäki, V., Mezger, M.

Physical Chemistry Chemical Physics, 21(7):3734-3741, Royal Society of Chemistry, Cambridge, England, 2019 (article)

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Connections Matter: On the Importance of Pore Percolation for Nanoporous Supercapacitors

Vasilyev, O., Kornyshev, A. A., Kondrat, S.

ACS Applied Energy Materials, 2(8):5386-5390, American Chemical Society, Washington, DC, 2019 (article)

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Theory of light-activated catalytic Janus particles

Uspal, W. E.

The Journal of Chemical Physics, 150(11), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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Recovering superhydrophobicity in nanoscale and macroscale surface textures

Giacomello, A., Schimmele, L., Dietrich, S., Tasinkevych, M.

Soft Matter, 15(37):7462-7471, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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Brownian dynamics assessment of enhanced diffusion exhibited by "fluctuating-dumbbell enzymes".

Kondrat, S., Popescu, M. N.

Physical Chemistry Chemical Physics, 21(35):18811-18815, Royal Society of Chemistry, Cambridge, England, 2019 (article)

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2017


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Chemically active colloids near osmotic-responsive walls with surface-chemistry gradients

Popescu, M. N., Uspal, W. E., Dietrich, S.

Journal of Physics: Condensed Matter, 29, IOP Publishing, Bristol, 2017 (article)

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2017


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Active colloids in the context of chemical kinetics

Oshanin, G., Popescu, M. N., Dietrich, S.

Journal of Physics A, 50, IOP Pub., Bristol, 2017 (article)

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Microbots Decorated with Silver Nanoparticles Kill Bacteria in Aqueous Media

Vilela, D., Stanton, M. M., Parmar, J., Sánchez, S.

ACS Applied Materials and Interfaces, 9(27):22093-22100, American Chemical Society, Washington, DC, 2017 (article)

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Measurement of second-order response without perturbation

Helden, L., Basu, U., Krüger, M., Bechinger, C.

EPL, 116(6), IOP Publishing, Bristol, 2017 (article)

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Swimming with a cage: low-Reynolds-number locomotion inside a droplet

Reigh, S., Zhu, L. L., Gallaire, F., Lauga, E.

Soft Matter, 13(17):3161-3173, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

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Active Particle Accumulation at Boundaries: A Strategy to Measure Contact Angles

Simmchen, J., Malgaretti, P.

ChemNanoMat, 3(11):790-793, Wiley, Weinheim, 2017 (article)

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Two-fluid model for locomotion under self-confinement

Reigh, S., Lauga, E.

Physical Review Fluids, 2(9), American Physical Society, 2017 (article)

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Bubble gating in biological ion channels: A density functional theory study

Gu\ssmann, Florian, Roth, R.

Physical Review E, 95(6), American Physical Society, Melville, NY, 2017 (article)

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Nematic films at chemically structured surfaces

Silvestre, N. M., Telo da Gama, M. M., Tasinkevych, M.

Journal of Physics: Condensed Matter, 29(7), IOP Publishing, Bristol, 2017 (article)

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