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2011


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Quantum-Cascade Laser-Based Vibrational Circular Dichroism

Luedeke, S., Pfeifer, M., Fischer, P.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 133(15):5704-5707, 2011 (article)

Abstract
Vibrational circular dichroism (VCD) spectra were recorded with a tunable external-cavity quantum-cascade laser (QCL). In comparison with standard thermal light sources in the IR, QCLs provide orders of magnitude more power and are therefore promising for VCD studies in strongly absorbing solvents. The brightness of this novel light source is demonstrated with VCD and IR absorption measurements of a number of compounds, including proline in water.

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DOI [BibTex]

2011


DOI [BibTex]


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Actively coupled cavity ringdown spectroscopy with low-power broadband sources

Petermann, C., Fischer, P.

OPTICS EXPRESS, 19(11):10164-10173, 2011 (article)

Abstract
We demonstrate a coupling scheme for cavity enhanced absorption spectroscopy that makes use of an intracavity acousto-optical modulator to actively switch light into (and out of) a resonator. This allows cavity ringdown spectroscopy (CRDS) to be implemented with broadband nonlaser light sources with spectral power densities of less than 30 mu W/nm. Although the acousto-optical element reduces the ultimate detection limit by introducing additional losses, it permits absorptivities to be measured with a high dynamic range, especially in lossy environments. Absorption measurements for the forbidden transition of gaseous oxygen in air at similar to 760nm are presented using a low-coherence cw-superluminescent diode. The same setup was electronically configured to cover absorption losses from 1.8 x 10(-8)cm(-1) to 7.5\% per roundtrip. This could be of interest in process analytical applications. (C) 2011 Optical Society of America

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DOI [BibTex]

DOI [BibTex]


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Magnetically actuated propulsion at low Reynolds numbers: towards nanoscale control

Fischer, P., Ghosh, A.

NANOSCALE, 3(2):557-563, 2011 (article)

Abstract
Significant progress has been made in the fabrication of micron and sub-micron structures whose motion can be controlled in liquids under ambient conditions. The aim of many of these engineering endeavors is to be able to build and propel an artificial micro-structure that rivals the versatility of biological swimmers of similar size, e. g. motile bacterial cells. Applications for such artificial ``micro-bots'' are envisioned to range from microrheology to targeted drug delivery and microsurgery, and require full motion-control under ambient conditions. In this Mini-Review we discuss the construction, actuation, and operation of several devices that have recently been reported, especially systems that can be controlled by and propelled with homogenous magnetic fields. We describe the fabrication and associated experimental challenges and discuss potential applications.

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Video - Nanospropellers DOI [BibTex]


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The Oxidation of Fe(111)

Davies, R., Edwards, D., Gräfe, J., Gilbert, L., Davies, P., Hutchings, G., Bowker, M.

Surface Science, 605(17-18):1754-1762, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Weak value amplified optical activity measurements

Pfeifer, M., Fischer, P.

Opt. Express, 19(17):16508-16517, OSA, 2011 (article)

Abstract
We present a new form of optical activity measurement based on a modified weak value amplification scheme. It has recently been shown experimentally that the left- and right-circular polarization components refract with slightly different angles of refraction at a chiral interface causing a linearly polarized light beam to split into two. By introducing a polarization modulation that does not give rise to a change in the optical rotation it is possible to differentiate between the two circular polarization components even after post-selection with a linear polarizer. We show that such a modified weak value amplification measurement permits the sign of the splitting and thus the handedness of the optically active medium to be determined. Angular beam separations of Δθ ∼ 1 nanoradian, which corresponds to a circular birefringence of Δn ∼ 1 × 10−9, could be measured with a relative error of less than 1%.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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High-resolution x-ray absorption spectroscopy of BaTiO_3: Experiment and first-principles calculations

Chassé, A., Borek, S., Schindler, K., Trautmann, M., Huth, M., Steudel, F., Makhova, L., Gräfe, J., Denecke, R.

Physical Review B, 84, pages: 195135, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Electron theory of fast and ultrafast dissipative magnetization dynamics

Fähnle, M., Illg, C.

{Journal of Physics: Condensed Matter}, 23, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Large-area hard magnetic L10-FePt nanopatterns by nanoimprint lithography

Bublat, T., Goll, D.

{Nanotechnology}, 22(31), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Hydrogen storage by cryoadsorption in ultrahigh-porosity metal-organic frameworks

Hirscher, M.

{Angewandte Chemie International Edition}, 50(3):581-582, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Multilayer Fresnel zone plate for soft X-ray microscopy resolves sub-39 nm structures

Mayer, M., Grévent, C., Szeghalmi, A., Knez, M., Weigand, M., Rehbein, S., Schneider, G., Baretzky, B., Schütz, G.

{Ultramicroscopy}, 111, pages: 1706-1711, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Generalized Gilbert equation including inertial damping: derivation from an extended breathing Fermi surface model

Fähnle, M., Steiauf, D., Illg, C.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]


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Hydrogen physisorption in high SSA microporous materials - A comparison between AX-21\textunderscore33 and MOF-177 at cryogenic conditions

Schlichtenmayer, M., Streppel, B., Hirscher, M.

{International Journal of Hydrogen Energy}, 36, pages: 586-591, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic vortex core reversal by excitation of spin waves

Kammerer, M., Weigand, M., Curcic, M., Noske, M., Sproll, M., Vansteenkiste, A., Van Waeyenberge, B., Stoll, H., Woltersdorf, G., Back, C. H., Schütz, G.

{Nature Communications}, 2, pages: 279-284, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetism studied with circularly polarized X-rays

Schütz, G., Goering, E., Stoll, H.

{International Journal of Materials Research}, 102(7):773-783, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Coupled vortex oscillations in spatially separated permalloy squares

Vogel, A., Kamionka, T., Martens, M., Drews, A., Chou, K., Tyliszczak, T., Stoll, H., Van Waeyenberge, B., Meier, G.

{Physical Review Letters}, 106, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Contruction of basis functions with crystal symmetry for the spin-cluster expansion of the magnetic energy on the atomic scale

Dietermann, F., Singer, R., Fähnle, M.

{Journal of Mathematical Physics}, 52, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic patterning perpendicular anisotropy FePd alloy films by masked ion irradiation

Merkel, D. G., Bottyán, L., Tanczikó, F., Zolnai, Z., Nagy, N., Vértesy, G., Waizinger, J., Bommer, L.

{Journal of Applied Physics}, 109(12), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Characterization of hydrogen/deuterium adsorption sites in nanoporous Cu-BTC by low-temperature thermal-desorption mass spectroscopy

Krkljus, I., Hirscher, M.

{Microporous and Mesoporous Materials}, 142, pages: 725-729, 2011 (article)

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DOI [BibTex]


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Stability of the current-carrying state in nonhomogeneous MgB2 films

Treiber, S., Stahl, C., Schütz, G., Albrecht, J.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Orbital reflectometry of oxide heterostructures

Benckiser, E., Haverkort, M. W., Brück, S., Goering, E., Macke, S., Fraño, A., Yang, X., Andersen, O. K., Cristiani, G., Habermeier, H., Boris, A. V., Zegkinoglou, I., Wochner, P., Kim, H., Hinkov, V., Keimer, B.

{Nature Materials}, 10(3):189-193, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Potential explanation of charge response of magnetization in nanoporous systems

Subkow, S., Fähnle, M.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Large hidden orbital moments in magnetite

Goering, E.

{Physica Status Solidi B}, 248(10):2345-2351, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Cr magnetization reversal at the CrO2/RuO2 interface: Origin of the reduced GMR effect

Zafar, K., Audehm, P., Schütz, G., Goering, E., Pathak, M., Chetry, K. B., LeClair, P. R., Gupta, A.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetocaloric effect, magnetic domain structure and spin-reorientation transitios in HoCo5 single crystals

Skokov, K. P., Pastushenkov, Y. G., Koshkid\textquotesingleko, Y. S., Schütz, G., Goll, D., Ivanova, T. I., Nikitin, S. A., Semenova, E. M., Petrenko, A. V.

{Journal of Magnetism and Magnetic Materials}, 323(5):447-450, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Elucidating gating effects for hydrogen sorption in MFU-4-type triazolate-based metal-organic frameworks featuring different pore sizes

Denysenko, D., Grzywa, M., Tonigold, M., Streppel, B., Krkljus, I., Hirscher, M., Mugnaioli, E., Kolb, U., Hanss, J., Volkmer, D.

{Chemistry - A European Journal}, 17(6):1837-1848, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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BET specific surface area and pore structure of MOFs determined by hydrogen adsorption at 20 K

Streppel, B., Hirscher, M.

{Physical Chemistry Chemical Physics}, 13(8):3220-3222, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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High contrast magnetic and nonmagnetic sample current microscopy for bulk and transparent samples using soft X-rays

Nolle, D., Weigand, M., Schütz, G., Goering, E.

{Microscopy and Microanalysis}, 17, pages: 834-842, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic vortex core reversal by rotating magnetic fields generated on micrometer length scales

Curcic, M., Stoll, H., Weigand, M., Sackmann, V., Jüllig, P., Kammerer, M., Noske, M., Sproll, M., Van Waeyenberge, B., Vansteenkiste, A., Woltersdorf, G., Tyliszczak, T., Schütz, G.

{Physica Status Solidi B}, 248(10):2317-2322, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Formation of two amorphous phases in the Ni60Nb18Y22 alloy after high pressure torsion

Straumal, B. B., Mazilkin, A. A., Protasova, S. G., Goll, D., Baretzky, B., Bakai, A. S., Dobatkin, S. V.

{Kovove Materialy-Metallic Materials}, 49(1):17-22, 2011 (article)

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link (url) [BibTex]

link (url) [BibTex]


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Structure and properties of nanograined Fe-C alloys after severe plastic deformation

Straumal, B. B., Dobatkin, S. V., Rodin, A. O., Protasova, S. G., Mazilkin, A. A., Goll, D., Baretzky, B.

{Advanced Engineering Materials}, 13(6):463-469, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Increased flux pinning in YBa2Cu3O7-δthin-film devices through embedding of Au nano crystals

Katzer, C., Schmidt, M., Michalowski, P., Kuhwald, D., Schmidl, F., Grosse, V., Treiber, S., Stahl, C., Albrecht, J., Hübner, U., Undisz, A., Rettenmayr, M., Schütz, G., Seidel, P.

{Europhysics Letters}, 95(6), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Signal transfer in a chain of stray-field coupled ferromagnetic squares

Vogel, A., Martens, M., Weigand, M., Meier, G.

{Applied Physics Letters}, 99, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Electron theory of magnetoelectric effects in metallic ferromagnetic nanostructures

Subkow, S., Fähnle, M.

{Physical Review B}, 84, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic antivortex-core reversal by rotating magnetic fields

Kamionka, T., Martens, M., Chou, K., Drews, A., Tyliszczak, T., Stoll, H., Van Waeyenberge, B., Meier, G.

{Physical Review B}, 83, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic properties of exchange-spring composite films

Kronmüller, H., Goll, D.

{Physica Status Solidi B}, 248(10):2361-2367, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Wetting transition of grain boundaries in the Sn-rich part of the Sn-Bi phase diagram

Yeh, C.-H., Chang, L.-S., Straumal, B. B.

{Journal of Materials Science}, 46(5):1557-1562, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Influence of dot size and annealing on the magnetic properties of large-area L10-FePt nanopatterns

Bublat, T., Goll, D.

{Journal of Applied Physics}, 110(7), 2011 (article)

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DOI [BibTex]


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The temperature-dependent magnetization profile across an epitaxial bilayer of ferromagnetic La2/3Ca1/3MnO3 and superconducting YBa2Cu3O7-δ

Brück, S., Treiber, S., Macke, S., Audehm, P., Christiani, G., Soltan, S., Habermeier, H., Goering, E., Albrecht, J.

{New Journal of Physics}, 13(3), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Spin interactions in bcc and fcc Fe beyond the Heisenberg model

Singer, R., Dietermann, F., Fähnle, M.

{Physical Review Letters}, 107, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Route to a family of robust, non-interpenetrated metal-organic frameworks with pto-like topology

Klein, N., Senkovska, I., Baburin, I. A., Grünker, R., Stoeck, U., Schlichtenmayer, M., Streppel, B., Mueller, U., Leoni, S., Hirscher, M., Kaskel, S.

{Chemistry - A European Journal}, 17(46):13007-13016, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Initial stages of growth of iron on silicon for spin injection through Schottky barrier

Dash, S. P., Carstanjen, H. D.

{Physica Status Solidi B}, 248(10):2300-2304, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Fe3O4/ZnO: A high-quality magnetic oxide-semiconductor heterostructure by reactive deposition

Paul, M., Kufer, D., Müller, A., Brück, S., Goering, E., Kamp, M., Verbeeck, J., Tian, H., Van Tendeloo, G., Ingle, N. J. C., Sing, M., Claessen, R.

{Applied Physics Letters}, 98, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Influence of texture on the ferromagnetic properties of nanograined ZnO films

Straumal, B., Mazilkin, A., Protasova, S., Myatiev, A., Straumal, P., Goering, E., Baretzky, B.

{Physica Status Solidi B}, 248(7):1581-1586, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Control of spin configuration in half-metallic La0.7Sr0.3MnO3 nano-structures

Rhensius, J., Vaz, C. A. F., Bisig, A., Schweitzer, S., Heidler, J., Körner, H. S., Locatelli, A., Niño, M. A., Weigand, M., Méchin, L., Gaucher, F., Goering, E., Heyderman, L. J., Kläui, M.

{Applied Physics Letters}, 99(6), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Comparison of various sol-gel derived metal oxide layers for inverted organic solar cells

Oh, H., Krantz, J., Litzov, I., Stubhan, T., Pinna, L., Brabec, C. J.

{Solar Energy Materials \& Solar Cells}, 95(8):2194-2199, 2011 (article)

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DOI [BibTex]

DOI [BibTex]

2000


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Phenomenological damping in optical response tensors

Buckingham, A., Fischer, P.

PHYSICAL REVIEW A, 61(3), 2000 (article)

Abstract
Although perturbation theory applied to the optical response of a molecule or material system is only strictly valid far from resonances, it is often applied to ``near-resonance{''} conditions by means of complex energies incorporating damping. Inconsistent signs of the damping in optical response tensors have appeared in the recent literature, as have errors in the treatment of the perturbation by a static held. The ``equal-sign{''} convention used in a recent publication yields an unphysical material response, and Koroteev's intimation that linear electro-optical circular dichroism may exist in an optically active liquid under resonance conditions is also flawed. We show that the isotropic part of the Pockels tensor vanishes.

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DOI [BibTex]

2000


DOI [BibTex]


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Ab initio investigation of the sum-frequency hyperpolarizability of small chiral molecules

Champagne, B., Fischer, P., Buckingham, A.

CHEMICAL PHYSICS LETTERS, 331(1):83-88, 2000 (article)

Abstract
Using a sum-over-states procedure based on configuration interaction singles /6-311++G{*}{*}, we have computed the sum-frequency hyperpolarizability beta (ijk)(-3 omega; 2 omega, omega) Of two small chiral molecules, R-monofluoro-oxirane and R-(+)-propylene oxide. Excitation energies were scaled to fit experimental UV-absorption data and checked with ab initio values from time-dependent density functional theory. The isotropic part of the computed hyperpolarizabilities, beta(-3 omega; 2 omega, omega), is much smaller than that reported previously from sum-frequency generation experiments on aqueous solutions of arabinose. Comparison is made with a single-centre chiral model. (C) 2000 Elsevier Science B.V. All rights reserved.

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DOI [BibTex]

DOI [BibTex]


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Three-wave mixing in chiral liquids

Fischer, P., Wiersma, D., Righini, R., Champagne, B., Buckingham, A.

PHYSICAL REVIEW LETTERS, 85(20):4253-4256, 2000 (article)

Abstract
Second-order nonlinear optical frequency conversion in isotropic systems is only dipole allowed for sum- and difference-frequency generation in chiral media. We develop a single-center chiral model of the three-wave mixing (sum:frequency generation) nonlinearity and estimate its magnitude. We also report results from ab initio calculations and from three- and four-wave mixing experiments in support of the theoretical estimates. We show that the second-order susceptibility in chiral liquids is much smaller than previously thought.

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DOI [BibTex]

DOI [BibTex]


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Anisotropic flux pinning in thin YBCO-films by substrate modifications

Leonhardt, S., Warthmann, R., Albrecht, J., Jooss, C., Kronmüller, H., Haage, T., Zegenhagen, J., Habermeier, H.-U.

{Physica C}, 332, pages: 214-218, 2000 (article)

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[BibTex]

[BibTex]